Klotsa, D. and Jack, R. L., 2011. Predicting the self-assembly of a model colloidal crystal. Soft Matter, 7 (13), pp. 6294-6303.
We investigate the self-assembly (crystallisation) of particles with hard cores and isotropic, square-well interactions, using a Monte Carlo scheme to simulate overdamped Langevin dynamics. We measure correlation and response functions during the early stages of assembly, and we analyse the results using fluctuation-dissipation theorems, aiming to predict which systems will self-assemble successfully and which will get stuck in disordered states. The early-time correlation and response measurements are made before significant crystallisation has taken place, indicating that dynamical measurements are valuable in measuring a system's propensity for kinetic trapping.
|Item Type ||Articles|
|Creators||Klotsa, D.and Jack, R. L.|
|Departments||Faculty of Science > Physics|
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